By Douglas C. Neckers, William S. Jenks, Thomas Wolff
Content material: Ensemble Photophysics of inflexible Polyphenylene established Dendritic buildings (M. Lor, G. Schweitzer, M. Van Der Auweraer, J. Hofkens, and F. C. De Schryver). Photochemistry of Short-Lived Species utilizing Multibeam Irradiation (Mamoru Fujitsuka and Tetsuro Majma). Two-Photon actual, natural, and Polymer Chemistry: concept, ideas, Chromophore layout, and purposes (Bernd Strehmel and Veronika Strehmel). Index. Cumulative Index Volumes
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Campagna, S. Serroni, M. Ciano, A. Juris, and V. Balzani, Inorg. Chem. 1992, 31, 2982. (b) V. Balzani, A. Juris, M. Venturi, S. Campagna, and S. Serroni, Chem. Rev. 1996, 96, 759. G. Bergamini, P. Ceroni, M. Maestri, V. -K. Lee, and F. Vo¨ gtle, Photochem. Photobiol. Sci. 2004, 3, 898. (a) S. Gilat, A. Adronov, and J. M. J. Fre´ chet, Angew. Chem. Int. Ed. 1999, 38, 1422. (b) A. Adronov, S. L. Gilat, J. M. J. Fre´ chet, K. Ohta, F. V. R. Neuwahl, and G. R. Fleming, J. Am. Chem. Soc. 2000, 122, 1175.
P. Ghiggino, J. N. H. Reek, M. J. Crossley, A. W. Bosman, A. P. H. J. Schenning, and E. W. Meijer, J. Phys. Chem. B 2000, 104, 2596. 15. (a) O. Varnavski, G. Menkir, and T. Goodson III, Appl. Phys. Lett. 2000, 77, 1120. (b) T. Goodson III, Acc. Chem. Res. 2005, 38, 99. 16. B. K. Kaletas, R. Dobrawa, A. Sautter, F. Wu¨ rthner, M. Zimine, L. De Cola, and R. M. Williams, J. Phys. Chem. A 2004, 108, 1900. 17. (a) S. Jordens, G. De Belder, M. Lor, G. Schweitzer, M. van der Auweraer, T. Weil, E. Reuther, K.
Using Eq. 85 nsÀ1 for khopp is obtained for these dendrimers. This value is more than five times smaller than that of the corresponding first generation dendrimers. 7 for k2 and khopp the distance between the two chromophores have been calculated from Eq. (6). This yields a value of d ¼ 3:7 nm, which is in good agreement with the average interchromophoric distance obtained from molecular modeling. 7 nm. 15, the multichromophoric second generation dendrimer is still inside the active sphere in which energy hopping can take place with high efficiencies.
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